Try the following:
this.chart1.BackColor = Color.AliceBlue;
this.chart1.ChartAreas[0].AxisX.LineColor = Color.Red;
this.chart1.ChartAreas[0].AxisX.MajorGrid.LineColor = Color.Red;
this.chart1.ChartAreas[0].AxisX.LabelStyle.ForeColor = Color.Red;
this.chart1.ChartAreas[0].AxisY.LineColor = Color.Red;
this.chart1.ChartAreas[0].AxisY.MajorGrid.LineColor = Color.Red;
this.chart1.ChartAreas[0].AxisY.LabelStyle.ForeColor = Color.Red;
This LabelStyle.ForeColorchanges the color of the label as you requested.
Properties LineColorand MajorGrid.LineColorallow you to change the grid lines (black in the screenshot), if you need it. Of course, the colors Red and AliceBlue are, for example.
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